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To assemble your cakes, spoon or pipe the mousse into silicone molds, not quite all the way full. Gently press a gelée sphere, curved side down, into the top of each mousse-filled mold. Scrape with an offset spatula to make the top perfectly level with the top of the mold.
Rinse a 4-cup mold with ice water. Scrape the mixture into the mold. Cover and refrigerate until set, several hours or overnight. To unmold, briefly dip mold once or twice into a bowl of hot water. Invert onto serving plate.
With mixer on low speed, pour in chocolate, making sure chocolate falls into the cream mixture, rather than hitting the side of the bowl. Mix just until incorporated. Rinse a 4-cup mold with ice water. Scrape the mixture into the mold. Cover and refrigerate until set, several hours or overnight.
The cakes use these small half-dome molds which are about 1 3/4″ in diameter (and the gelée is molded with the mini size). You could also use a larger semi-sphere mold for your cakes (and I admit, these are definitely less than a single serving worth).
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